为此,有也人们开发了几种合成方法来制备2DMOF薄膜。(2)团队在该领域工作汇总[1]Y. Liu,天生Y. Wei,天生M. Liu,Y. Bai,X. Wang,S. Shang,J. Chen*,Y. Liu*,ElectrochemicalSynthesisofLargeAreaTwo‐DimensionalMetal–OrganicFrameworkFilmsonCopperAnodes,Angew.Chem.Int.Ed.2021, 133,2923[2]X. Du,J. Zhang,H. Wang,Z. Huang,A. Guo,L. Zhao,Y. Niu,I. Li,B. Wu*andY. Liu*, Solid-solidinterfacegrowthofconductivemetal-organicframeworknanowirearraysandtheirsupercapacitorapplication, Mater.Chem.Front. 2020, 4,243-251.[3]X. Chen,#H. Yang,#B. Wu,*L. Wang,Q. Fu,andY. Liu*,EpitaxialGrowthofh-BNonTemplatesofVariousDimensionalitiesinh-BN–grapheneMaterialSystems, Adv. Mater. 2019,31, 1805582.[4]L. Fu,D. Hu,RafaelG.Mendes,MarkH.Rümmeli,Q. Dai,B. Wu,*L. Fu,*andY. Liu,*HighlyOrganizedEpitaxyofDiracSemimetallicPtTe2CrystalswithExtrahighConductivityandVisibleSurfacePlasmonsatEdges, ACS Nano, 2018,12,9405-9411.[5]L. Fu,F. Wang,B. Wu,*N. Wu,W. Huang,H. Wang,C. Jin,L. Zhuang,J. He,L. Fu,*andY. Liu* VanderWaalsEpitaxialGrowthofAtomicLayeredHfS2CrystalsforUltrasensitiveNear-InfraredPhototransistors, Adv. Mater. 2017,29,1700439.(3)相关优质文献推荐[1]X.Song,X.Wang,Y.Li,C.Zheng,B.Zhang,C.-a.Di,F.Li,C.Jin,W.Mi,L.Chen,W.Hu,2DSemiconductingMetal-OrganicFrameworkThinFilmsfor OrganicSpinValves,Angew.Chem.Int.Ed. 2020,59,1118.[2]M.-S.Yao,X.-J.Lv,Z.-H.Fu,W.-H.Li,W.-H.Deng,G.-D.Wu,G.Xu,Layer-by-LayerAssembledConductiveMetal–OrganicFramework NanofilmsforRoom-TemperatureChemiresistiveSensing,Angew.Chem.Int.Ed. 2017,56,16510.[3]VitalieStavila, JoanneVolponi, AaronM.Katzenmeyer, MatthewC.Dixonb,MarkD.Allendorf,Kineticsandmechanismofmetal–organicframeworkthinfilmgrowth:systematicinvestigationofHKUST-1depositiononQCMelectrodes,Chem.Sci. 2012,3,1531.[4]MonicaC.So,ShengyeJin,Ho-JinSon,GaryP.Wiederrecht,OmarK.Farha,JosephT.Hupp,Layer-by-LayerFabricationofOrientedPorousThinFilmsBasedonPorphyrin-ContainingMetal−OrganicFrameworks, J.Am.Chem.Soc. 2013,135,42,15698[5]JinxuanLiu,ChristofWöll,Surface-supportedmetal–organicframeworkthinfilms:fabricationmethods,applications,andchallenges, Chem.Soc.Rev. 2017,46,5730.本文由木文韬翻译,材料牛整理编辑。终点c)器件在N2气氛下的Ids-Vds曲线。
该策略同样也适用于制备其他晶圆级导电MOF薄膜如M3(HHTP)2(M=Cu、有也Co和Ni。欢迎大家到材料人宣传科技成果并对文献进行深入解读,天生投稿邮箱[email protected]。
终点e)升降温过程中器件的归一化电导(σ)变化(A:温度/K。
近年来,有也人们合成了一系列导电MOF薄膜,并将其应用于传感器、电池电极、超导体等电子活性层。最近的研究表明,天生在熔融金表面或块状铜箔上单晶hBN薄膜的生长。
先前在Cu(111)金属上生长hBN单层的尝试未能实现单取向,终点当这些层合并成flms时会导致有害的晶界。有也2D半导体的一个主要挑战是避免从相邻的电介质形成电荷散射和捕获位点。
天生文献链接:Acoatingfromnature.(Sci.Adv.,2020,DOI:10.1126/sciadv.abe0026)8.三星先进研究院NatureEnergy:银碳复合阳极可实现高能长循环全固态锂金属电池具有锂金属阳极的全固态电池是超越常规锂离子电池性能的强大选择。近来,终点已经在高压下的几种系统中报道了富氢材料中的高温常规超导性。